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Abstract Spin-orbit coupled honeycomb magnets with the Kitaev interaction have received a lot of attention due to their potential of hosting exotic quantum states including quantum spin liquids. Thus far, the most studied Kitaev systems are 4 d /5 d -based honeycomb magnets. Recent theoretical studies predicted that 3 d -based honeycomb magnets, including Na 2 Co 2 TeO 6 (NCTO), could also be a potential Kitaev system. Here, we have used a combination of heat capacity, magnetization, electron spin resonance measurements alongside inelastic neutron scattering (INS) to study NCTO’s quantum magnetism, and we have found a field-induced spin disordered state in an applied magnetic field range of 7.5 T < B (⊥ b -axis) < 10.5 T. The INS spectra were also simulated to tentatively extract the exchange interactions. As a 3 d -magnet with a field-induced disordered state on an effective spin-1/2 honeycomb lattice, NCTO expands the Kitaev model to 3 d compounds, promoting further interests on the spin-orbital effect in quantum magnets.more » « less
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Tian, Long ; Liu, Panpan ; Xu, Zhuang ; Li, Yu ; Lu, Zhilun ; Walker, H. C. ; Stuhr, U. ; Tan, Guotai ; Lu, Xingye ; Dai, Pengcheng ( , Physical Review B)
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Balz, Christian ; Lampen-Kelley, Paula ; Banerjee, Arnab ; Yan, Jiaqiang ; Lu, Zhilun ; Hu, Xinzhe ; Yadav, Swapnil M. ; Takano, Yasu ; Liu, Yaohua ; Tennant, D. Alan ; et al ( , Physical Review B)